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An integrated approach for machine-learning-based system identification of dynamical systems under control: application towards the model predictive control of a highly nonlinear reactor system

《化学科学与工程前沿（英文）》 2022年 第16卷 第2期   页码 237-250 doi: 10.1007/s11705-021-2058-6

摘要： Advanced model-based control strategies, e.g., model predictive control, can offer superior control of key process variables for multiple-input multiple-output systems. The quality of the system model is critical to controller performance and should adequately describe the process dynamics across its operating range while remaining amenable to fast optimization. This work articulates an integrated system identification procedure for deriving black-box nonlinear continuous-time multiple-input multiple-output system models for nonlinear model predictive control. To showcase this approach, five candidate models for polynomial and interaction features of both output and manipulated variables were trained on simulated data and integrated into a nonlinear model predictive controller for a highly nonlinear continuous stirred tank reactor system. This procedure successfully identified system models that enabled effective control in both servo and regulator problems across wider operating ranges. These controllers also had reasonable per-iteration times of ca. 0.1 s. This demonstration of how such system models could be identified for nonlinear model predictive control without prior knowledge of system dynamics opens further possibilities for direct data-driven methodologies for model-based control which, in the face of process uncertainties or modelling limitations, allow rapid and stable control over wider operating ranges.

关键词： nonlinear model predictive control     black-box modeling     continuous-time system identification     machine learning     industrial applications of process control    

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针对下肢外骨骼机器人的基于概率运动基元的黑盒优化运动学习 Research Article

王嘉琪,高永卓,吴冬梅,董为

《信息与电子工程前沿（英文）》 2023年 第24卷 第1期   页码 104-116 doi: 10.1631/FITEE.2200065

摘要： 外骨骼作为一种可穿戴的机器人，通过拟人化的构型直接传递机械动力来辅助或增强穿戴者运动。当外骨骼用于促进穿戴者的运动时，运动生成过程通常在高层控制中发挥重要作用。该领域的主要挑战之一是实时生成符合人类意图且可以适应不同情况的参考轨迹。在本文中，我们首先提出了一种基于概率运动基元（ProMP）的下肢外骨骼运动建模方法，它是一种用于生成运动轨迹的新型且强大的代表性工具。为了在不同穿戴者使用外骨骼时使轨迹适应不同情况，我们接着提出了一种基于黑盒优化PIBB结合ProMP的新型运动学习方案。运动模型首先由ProMP离线学习，它可以生成参考轨迹供外骨骼控制器在线使用，再采用PIBB在线学习和更新模型，提供了系统的自适应能力，消除了不确定性的影响。使用下肢外骨骼HEXO对六名受试者进行的模拟和实验证明了所提出方法的有效性。

关键词： 下肢外骨骼机器人；人机交互；运动学习；轨迹生成；运动基元；黑盒优化    

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针对工业故障分类系统的单变量攻击及其防御 Article

卓越, Yuri A.W. Shardt, 葛志强

《工程（英文）》 2022年 第19卷 第12期   页码 240-251 doi: 10.1016/j.eng.2021.07.033

摘要：

近年来，工业过程故障分类系统主要是由数据驱动的，得益于大量的数据模式，基于深度神经网络的模型显著地提高了故障分类的准确性。但是，这些数据驱动模型容易受到对抗攻击，因此，在样本上的微小扰动会导致模型提供错误的故障预测。最近的研究已经证明了机器学习模型的脆弱性以及对抗样本的广泛存在。本文针对安全、关键的工业故障分类系统提出了一种具有极端约束的黑盒攻击方法：只扰动一个变量来制作对抗样本。此外，为了将对抗样本隐藏在可视化空间中，本文使用了雅可比矩阵来引导扰动变量的选择，使降维空间中的对抗样本对人眼不可见。利用单变量攻击（OVA）方法，文本探究了不同工业变量和故障类别的脆弱性，有助于理解故障分类系统的几何特征。基于攻击方法，文本还提出了相应的对抗训练防御方法，该方法能够有效地防御单变量攻击，并提高分类器的预测精度。在实验中，将本文所提出的方法在田纳西-伊士曼过程（TEP）和钢板（SP）故障数据集上进行了测试。本文探索了变量和故障类别的脆弱相关性，并验证了各种分类器和数据集的单变量攻击和防御方法的有效性。对于工业故障分类系统，单变量攻击方法的攻击成功率接近（在TEP上）甚至高于（在SP 上）目前最有效的一阶白盒攻击方法（该方法需要对所有变量进行扰动）。

关键词： 对抗样本     黑盒攻击     工业数据安全     故障分类系统    

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Adsorption property of direct fast black onto acid-thermal modified sepiolite and optimization of adsorptionconditions using Box-Behnken response surface methodology

Chengyuan SU, Weiguang LI, Yong WANG

《环境科学与工程前沿（英文）》 2013年 第7卷 第4期   页码 503-511 doi: 10.1007/s11783-012-0477-9

摘要： The adsorption of direct fast black onto acid-thermal modified sepiolite was investigated. Batch adsorption experiments were performed to evaluate the influences of experimental parameters such as initial dye concentration, initial solution pH and adsorbent dosage on the adsorption process. The three-factor and three-level Box-Behnken response surface methodology (RSM) was utilized for modeling and optimization of the adsorption conditions for direct fast black onto the acid-thermal modified sepiolite. The raw sepiolite was converted to acid-thermal modified sepiolite, and changes in the fourier transform infrared spectrum (FTIR) adsorption bands of the sample were noted at 3435 cm and 1427 cm . The zeolitic water disappeared and the purity of sepiolite was improved by acid-thermal modification. The decolorization rate of direct fast black adsorbed increased from 68.2% to 98.9% on acid-thermal modified sepiolite as the initial solution pH decreased from 10 to 2. When the adsorbent dosage reached to 2.5 g·L , 2.0 g·L , 1.5 g·L and 1.0 g·L , the decolorization rate was 90.3%, 86.7%, 61.0% and 29.8%, respectively. When initial dye concentration increased from 25 to 200 mg·L , the decolorization rate decreased from 91.9% to 60.0%. The RSM results showed that the interaction between adsorbent dosage and pH to be a significant factor. The optimum conditions were as follows: the adsorbent dosage 1.99 g·L , pH 4.22, and reaction time 5.2 h. Under these conditions, the decolorization rate was 95.1%. The three dimensional fluorescence spectra of direct fast black before and after treatment showed that the direct fast black was almost all adsorbed by the acid-thermal modified sepiolite.

关键词： direct fast black     acid-thermal modified sepiolite     adsorption     response surface methodology    

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Enhancement of the electrocatalytic oxidation of antibiotic wastewater over the conductive black carbon-PbO

Xiangyu Wang, Yu Xie, Guizhen Yang, Jiming Hao, Jun Ma, Ping Ning

《环境科学与工程前沿（英文）》 2020年 第14卷 第2期 doi: 10.1007/s11783-019-1201-9

摘要： • A novel conductive carbon black modified lead dioxide electrode is synthesized. • The modified PbO2 electrode exhibits enhanced electrochemical performances. • BBD method could predict optimal experiment conditions accurately and reliably. • The modified electrode possesses outstanding reusability and safety. The secondary pollution caused by modification of an electrode due to doping of harmful materials has long been a big concern. In this study, an environmentally friendly material, conductive carbon black, was adopted for modification of lead dioxide electrode (PbO2). It was observed that the as-prepared conductive carbon black modified electrode (C-PbO2) exhibited an enhanced electrocatalytical performance and more stable structure than a pristine PbO2 electrode, and the removal efficiency of metronidazole (MNZ) and COD by a 1.0% C-PbO2 electrode at optimal conditions was increased by 24.66% and 7.01%, respectively. Results revealed that the electrochemical degradation of MNZ wastewater followed pseudo-first-order kinetics. This intimates that the presence of conductive carbon black could improve the current efficiency, promote the generation of hydroxyl radicals, and accelerate the removal of MNZ through oxidation. In addition, MNZ degradation pathways through a C-PbO2 electrode were proposed based on the identified intermediates. To promote the electrode to treat antibiotic wastewater, optimal experimental conditions were predicted through the Box-Behnken design (BBD) method. The results of this study suggest that a C-PbO2 electrode may represent a promising functional material to pretreat antibiotic wastewaters.

关键词： Conductive carbon black     PbO2 electrode     Metronidazole     Electrochemical oxidation     Box-Behnken design-response surface method    

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Gray-box modeling and QFT control for precision servo transmission systems

Xiulan BAO, Xuedong CHEN, Xin LUO, Haocheng ZUO

《机械工程前沿（英文）》 2011年 第6卷 第4期   页码 442-448 doi: 10.1007/s11465-011-0242-y

摘要：

Precision servo transmission systems have widely been applied in industrial equipment to achieve high accuracy and high speed motion. However, due to the presence of friction and uncertainty, the characteristics of precision servo transmission systems are variant depends on the working conditions, leading to oscillation and instability in the system performances. In this paper, a grey-box model of the system is established, the model structure derived from the theoretical modeling and the model parameters are obtained by experiments using set membership identification method. This paper proposes two-degrees of freedom (2-DOF) robust position controller for a precision servo transmission system, based on the quantitative feedback theory (QFT), to achieve high accuracy and consistent tracking performance even in presence of considerable system uncertainties and friction disturbances. The results of simulate and experiment validate the effectiveness of the proposed controller.

关键词： precision servo transmission system     modeling     set membership identification     quantitative feedback theory (QFT)     robustness    

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Preparation of nZVI embedded modified mesoporous carbon for catalytic persulfate to degradation of reactive black

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1372-4

摘要：

• The MCNZVI is prepared as an interesting material for PS activation.

关键词： MCNZVI     Core-shell structure     Reactive Black 5     Persulfate     Mechanism    

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Characteristics of typical dissolved black carbons and their influence on the formation of disinfection

《环境科学与工程前沿（英文）》 2022年 第16卷 第12期 doi: 10.1007/s11783-022-1585-9

摘要：

● The physicochemical and structural properties of DBC were characterized.

关键词： Dissolved black carbon (DBC)     Chlorine     Chloramine     Disinfection by-products (DBPs)     Disinfection by-products formation potential (DBPFP)    

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oxide for active and intelligent packaging: comparison of anthocyanins source from purple tomato or black

《化学科学与工程前沿（英文）》 2023年 第17卷 第6期   页码 704-715 doi: 10.1007/s11705-022-2270-z

摘要： The multifunctional films was prepared by blending chitosan and nano-ZnO with purple tomato anthocyanins or black wolfberry anthocyanins. The properties of films functioned by anthocyanins source and nano-ZnO content were studied. It was found purple tomato anthocyanins showed more significant color change against pH than black wolfberry anthocyanins. The nano-ZnO were widely dispersed in matrix and enhanced the compatibility of anthocyanins with chitosan. However, the anthocyanins source influenced the properties of the films more slightly than nano-ZnO addition. The tensile strength, antioxidant and antibacterial effects of the chitosan films dramatically increased after cooperated by nano-ZnO and anthocyanins, which also enhanced with increase of nano-ZnO content, whereas the elongation at break of the composite films decreased. Especially, the anthocyanin and nano-ZnO promoted the antibacterial activity of films synergistically. Composite films made from black wolfberry anthocyanins exhibited higher mechanical performance than those made from purple tomato anthocyanins but weaker antibacterial effects. The purple tomato anthocyanins/chitosan and nano-ZnO/purple tomato anthocyanins/chitosan films effectively reflected pork spoilage, changing their colors from dark green to brown, indicating the potential for applications in active and intelligent food packaging.

关键词： bio-based     multifunction     colorimetric indicator     active and intelligent packaging    

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Property-performance relationship of core-shell structured black TiO photocatalyst for environmental

《环境科学与工程前沿（英文）》 2023年 第17卷 第9期 doi: 10.1007/s11783-023-1711-3

摘要：

● Properties and performance relationship of CSBT photocatalyst were investigated.

关键词： Black TiO2     Core-shell structure     Property-performance relationship     Agro-industrial effluent     Environmental remediation    

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Effect of inlet box on performance of axial flow fans

LI Jingyin, TIAN Hua, YUAN Xiaofang

《能源前沿（英文）》 2008年 第2卷 第4期   页码 390-394 doi: 10.1007/s11708-008-0087-1

摘要： Numerical investigations on 3D flow fields in an axial flow fan with and without an inlet box have been extensively conducted, focusing on the variation of fan performance caused by the internal flow fields and the velocity evenness at the exit of the inlet box. It is interesting to find that although the inlet box is well designed in accordance with basic design principles, there is a flow separation region in it. Furthermore, this flow separation and the resulting uneven velocity distribution at the exit lead to some decrease in the efficiency and an increase in the total pressure rise of the fan. This research shows that the inlet box needs further improvement and such a check on the flow fields is of value for the design of inlet boxes.

关键词： box     velocity distribution     accordance     Numerical     variation    

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On subsurface box-shaped lined tunnel under incident SH-wave propagation

《结构与土木工程前沿（英文）》 2021年 第15卷 第4期   页码 948-960 doi: 10.1007/s11709-021-0740-x

摘要： In this paper, a half-plane time-domain boundary element method is applied to obtain the seismic ground response, including a subsurface box-shaped lined tunnel deployed in a linear homogenous elastic medium exposed to obliquely incident SH-waves. Only the boundary around the tunnel is required to be discretized. To prepare an appropriate model by quadratic elements, a double-node procedure is used to receive dual boundary fields at corners as well as change the direction of the normal vector. After encoding the method in a previously confirmed computer program, a numerical study is carried out to sensitize some effective parameters, including frequency content and incident wave angle for obtaining a surface response. The depth and impedance ratio of the lining are assumed to be unvaried. The responses are illustrated in the time and frequency domains as two/three-dimensional graphs. The results showed that subsurface openings with sharp corners distorted the propagation path of the anti-plane waves to achieve the critical states on the ground surface. The present approach can be proposed to civil engineers for preparing simple underground box-shaped models with angular boundaries.

关键词： box-lined tunnel     half-plane BEM     surface response     SH-wave     time-domain    

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Community diversity and distribution of ammonia-oxidizing archaea in marsh wetlands in the black soil

Chunhong Chen, Hong Liang, Dawen Gao

《环境科学与工程前沿（英文）》 2019年 第13卷 第4期 doi: 10.1007/s11783-019-1146-z

摘要：

AOA amoA genes in the soils of the two wetlands affiliated with three lineages.

The main drivers of AOA community were pH and total organic carbon and ammonium.

The soil characteristics rather than the vegetation control the AOA community.

关键词： Ammonia-oxidizing archaea     amoA gene     Freshwater marsh     Diversity     Distribution    

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Contribution of black carbon to nonlinearity of sorption and desorption of acetochlor on sediment

Jianqiu LIU, Yaobin ZHANG, Hong CHEN, Yazhi ZHAO, Xie QUAN

《环境科学与工程前沿（英文）》 2009年 第3卷 第1期   页码 69-74 doi: 10.1007/s11783-008-0076-y

摘要： In order to investigate the contribution of various black carbon (BC) contents to nonlinearity of sorption and desorption isotherms for acetochlor on sediment, equilibrium sorption and desorption isotherms were determined to measure sorption and desorption of acetochlor in sediment amended with various amounts of BC. In this paper, two types of BC referred to as BC400 and BC500 were prepared at 400°C and 500°C, respectively. Higher preparation temperature facilitated the formation of micropores on BC to enhance its sorption capacity. Increase of the BC content obviously increased the sorption amount and reduced the desorption amount for acetochlor. When the BC500 contents in total organic carbon (TOC) increased from 0 to 60%, Freundlich sorption coefficient ( ) increased from 4.07 to 35.74, and desorption hysteresis became gradually obvious. When the content of BC in TOC was lower than 23%, the sorption isotherm had a significant linear correlation ( = 0.05). In case of desorption, a significant nonlinear change could be observed when the content of BC was up to 13%. Increase of BC content in the sediment would result in shifting the sorption-desorption isotherms from linearity to nonlinearity, which indicated that contribution of BC to nonlinear adsorption fraction became gradually remarkable.

关键词： black carbon (BC)     sorption     desorption     sediment    

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Effect of carbon black on the dynamic moduli of asphalt mixtures and its master curves

Chuangmin LI, Fanbo NING, Yuanyuan LI

《结构与土木工程前沿（英文）》 2019年 第13卷 第4期   页码 918-925 doi: 10.1007/s11709-019-0526-6

摘要： Modulus is one of the main parameters during the design of asphalt pavement structure, the newest specifications of China gives the dynamic moduli ranges of commonly used asphalt mixtures with base asphalt (BA) or styrene-butadiene-styrene modified asphalt (SBS MA), while the moduli ranges of mixtures with carbon black modified asphalt (CB MA) are not recommended. To investigate the CB effect on the dynamic moduli of CB MA mixtures, one commonly used asphalt mixture (AC-20) was designed with BA, SBS MA, and CB MA, respectively. Then, the uniaxial compression dynamic modulus tests were conducted at different temperatures and loading frequencies, the master curves of asphalt mixtures were analyzed based on the time-temperature equivalence principle. The results show that ith increasing loading frequency, the temperature dependence of dynamic moduli of all asphalt mixtures tend to be less obvious. Both SBS and CB can decrease the temperature sensitivity of asphalt mixture, the SBS MA mixture has the lowest temperature sensitivity, followed by CB MA and BA mixture. In addition, CB and SBS can obviously improve the dynamic modulus of the BA mixture, enhance the anti-deformation performance of pavement structure, and the improvement effect of CB is almost the same with SBS.

关键词： dynamic modulus     carbon black     master curve     modified asphalt     asphalt mixture    

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标题 作者 时间 类型 操作

An integrated approach for machine-learning-based system identification of dynamical systems under control: application towards the model predictive control of a highly nonlinear reactor system

期刊论文

针对下肢外骨骼机器人的基于概率运动基元的黑盒优化运动学习

王嘉琪,高永卓,吴冬梅,董为

期刊论文

针对工业故障分类系统的单变量攻击及其防御

卓越, Yuri A.W. Shardt, 葛志强

期刊论文

Adsorption property of direct fast black onto acid-thermal modified sepiolite and optimization of adsorptionconditions using Box-Behnken response surface methodology

Chengyuan SU, Weiguang LI, Yong WANG

期刊论文

Enhancement of the electrocatalytic oxidation of antibiotic wastewater over the conductive black carbon-PbO

Xiangyu Wang, Yu Xie, Guizhen Yang, Jiming Hao, Jun Ma, Ping Ning

期刊论文

Gray-box modeling and QFT control for precision servo transmission systems

Xiulan BAO, Xuedong CHEN, Xin LUO, Haocheng ZUO

期刊论文

Preparation of nZVI embedded modified mesoporous carbon for catalytic persulfate to degradation of reactive black

期刊论文

Characteristics of typical dissolved black carbons and their influence on the formation of disinfection

期刊论文

oxide for active and intelligent packaging: comparison of anthocyanins source from purple tomato or black

期刊论文

Property-performance relationship of core-shell structured black TiO photocatalyst for environmental

期刊论文

Effect of inlet box on performance of axial flow fans

LI Jingyin, TIAN Hua, YUAN Xiaofang

期刊论文

On subsurface box-shaped lined tunnel under incident SH-wave propagation

期刊论文

Community diversity and distribution of ammonia-oxidizing archaea in marsh wetlands in the black soil

Chunhong Chen, Hong Liang, Dawen Gao

期刊论文

Contribution of black carbon to nonlinearity of sorption and desorption of acetochlor on sediment

Jianqiu LIU, Yaobin ZHANG, Hong CHEN, Yazhi ZHAO, Xie QUAN

期刊论文

Effect of carbon black on the dynamic moduli of asphalt mixtures and its master curves

Chuangmin LI, Fanbo NING, Yuanyuan LI

期刊论文